Oak Ridge Today

ORNL scientists uncover clues to role of magnetism in iron-based superconductors

Posted at
By Leave a Comment

Magnetism of Iron-based Superconductors

Oak Ridge National Laboratory scientists used scanning transmission electron microscopy to measure atomic-scale magnetic behavior in several families of iron-based superconductors. (Photo courtesy ORNL)

 

New measurements of atomic-scale magnetic behavior in iron-based superconductors by researchers at Oak Ridge National Laboratory and Vanderbilt University are challenging conventional wisdom about superconductivity and magnetism.

The study published in Advanced Materials provides experimental evidence that local magnetic fluctuations can influence the performance of iron-based superconductors, which transmit electric current without resistance at relatively high temperatures.

“In the past, everyone thought that magnetism and superconductivity could not coexist,” said ORNL’s Claudia Cantoni, the study’s first author. “The whole idea of superconductors is that they expel magnetic fields. But in reality things are more complicated.”

Superconductivity is strongly suppressed by the presence of long-range magnetism—where atoms align their magnetic moments over large volumes—but the ORNL study suggests that rapid fluctuations of local magnetic moments have a different effect. Not only does localized magnetism exist, but it is also correlated with a high critical temperature, the point at which the material becomes superconducting. [Read more…]

ORNL paper examines clues for superconductivity in an iron-based material

Posted at
By Leave a Comment

FERMI Figure

A change of Hall and Seebeck effects point to large Fermi surface modification at the structural transition, preventing superconductivity at low temperatures. The change in the Fermi surface topology has been confirmed by angle-resolved photoemission spectroscopy. (Image courtesy ORNL)

For the first time, scientists have a clearer understanding of how to control the appearance of a superconducting phase in a material, adding crucial fundamental knowledge and perhaps setting the stage for advances in the field of superconductivity.

The paper, published in Physical Review Letters, focuses on a calcium-iron-arsenide single crystal, which has structural, thermodynamic, and transport properties that can be varied through carefully controlled synthesis, similar to the application of pressure. To make this discovery, researchers focused on how these changes alter the material’s Fermi surface, which maps the specific population and arrangement of electrons in materials.

“The Fermi surface is basically the ‘genetic code’ for causing a certain property, including superconductivity, in a material,” said Athena Safa-Sefat of the U.S. Department of Energy’s Oak Ridge National Laboratory, which led the research team. “We can make different phases of this material in single crystal forms and measure their structure and properties, but now we have Fermi surface signatures that explain why we can’t induce superconductivity in a certain structural phase of this material.” [Read more…]